Single-exposure elemental differentiation and texture-sensitive phase-retrieval imaging with a neutron counting micro-channel plate detector

Micro-channel plate (MCP) detectors, when used at pulsed-neutron-source instruments, offer the possibility of high spatial resolution and high contrast imaging with pixel-level spectroscopic information. Here we demonstrate the possibility of multimodal analysis including total neutron cross-section spectra measurements, quantitative material differentiation imaging and texture-sensitive in-line phase imaging, from a single exposure using an MCP detector. This multimodal approach operates in full-field imaging mode, with the neutron transmission spectra acquired at each individual detector pixel. Due to the polychromatic nature of the beam and spectroscopic resolving capability of the detector, no energy scanning is required. Good agreement with the library reference data is demonstrated for neutron cross-section spectra measurements. Two different images corresponding to two selected energy bandwidths are used for elemental differentiation imaging. Moreover, the presence of changes in texture, i.e., preferred grain orientation, in the sample is identified from our phase-retrieval imaging results.

Universal mask for hard X rays

Multiple exposures, of a single illuminated non-configurable mask that is transversely displaced to a number of specified positions, can be used to create any desired distribution of radiant exposure. An experimental proof-of-concept is given for this idea, employing hard X rays. The method is termed "ghost projection", since it may be viewed as a reversed form of classical ghost imaging. The written pattern is arbitrary, up to a tunable constant offset, together with a limiting spatial resolution that is governed by the finest features present in the illuminated mask. The method, which is immune to both proximity-correction and aspect-ratio issues, can be used to make a universal lithographic mask in the hard-X-ray regime. Ghost projection may also be used as a dynamically-configurable beam-shaping element, namely the hard-X-ray equivalent of a spatial light modulator. The idea may be applied to other forms of radiation and matter waves, such as gamma rays, neutrons, electrons, muons, and atomic beams.

Paraxial diffusion-field retrieval

Unresolved spatially-random microstructure, in an illuminated sample, can lead to position-dependent blur when an image of that sample is taken using an incoherent imaging system. For a small propagation distance, between the exit surface of the sample and the entrance surface of a position-sensitive detector, the paraxial approximation implies that the blurring influence of the sample may be modeled using an anomalous-diffusion field. This diffusion field may have a scalar or tensor character, depending on whether the random microstructure has an autocorrelation function that is rotationally isotropic or anisotropic, respectively. Partial differential equations are written down and then solved, in a closed-form manner, for several variants of the inverse problem of diffusion-field retrieval given suitable intensity images. Both uniform-illumination and structured-illumination schemes are considered. Links are made, between the recovered diffusion field and certain statistical properties of the unresolved microstructure. The developed theory -- which may be viewed as a crudely parallel form of small-angle scattering under the Guinier approximation -- is applicable to a range of paraxial radiation and matter fields, such as visible light, x rays, neutrons, and electrons.

Optimizing illumination patterns for classical ghost imaging

Classical ghost imaging is a new paradigm in imaging where the image of an object is not measured directly with a pixelated detector. Rather, the object is subject to a set of illumination patterns and the total interaction of the object, e.g., reflected or transmitted photons or particles, is measured for each pattern with a single-pixel or bucket detector. An image of the object is then computed through the correlation of each pattern and the corresponding bucket value. Assuming no prior knowledge of the object, the set of patterns used to compute the ghost image dictates the image quality. In the visible-light regime, programmable spatial light modulators can generate the illumination patterns. In many other regimes -- such as x rays, electrons, and neutrons -- no such dynamically configurable modulators exist, and patterns are commonly produced by employing a transversely-translated mask. In this paper we explore some of the properties of masks or speckle that should be considered to maximize ghost-image quality, given a certain experimental classical ghost-imaging setup employing a transversely-displaced but otherwise non-configurable mask.

Ghost projection. II. Beam shaping using realistic spatially-random masks

The spatial light modulator and optical data projector both rely on precisely configurable optical elements to shape a light beam. Here we explore an image-projection approach which does not require a configurable beam-shaping element. We term this approach {\em ghost projection} on account of its conceptual relation to computational ghost imaging. Instead of a configurable beam shaping element, the method transversely displaces a single illuminated mask, such as a spatially-random screen, to create specified distributions of radiant exposure. The method has potential applicability to image projection employing a variety of radiation and matter wave fields, such as hard x rays, neutrons, muons, atomic beams and molecular beams. Building on our previous theoretical and computational studies, we here seek to understand the effects, sensitivity, and tolerance of some key experimental limitations of the method. Focusing on the case of hard x rays, we employ experimentally acquired masks to numerically study the deleterious effects of photon shot noise, inaccuracies in random-mask exposure time, and inaccuracies in mask positioning, as well as adapting to spatially non-uniform illumination. Understanding the influence of these factors will assist in optimizing experimental design and work towards achieving ghost projection in practice.

Tomographic phase and attenuation extraction for a sample composed of unknown materials using X-ray propagation-based phase-contrast imaging

Propagation-based phase-contrast X-ray imaging (PB-PCXI) generates image contrast by utilizing sample-imposed phase-shifts. This has proven useful when imaging weakly-attenuating samples, as conventional attenuation-based imaging does not always provide adequate contrast. We present a PB-PCXI algorithm capable of extracting the X-ray attenuation, $\beta$, and refraction, $\delta$, components of the complex refractive index of distinct materials within an unknown sample. The method involves curve-fitting an error-function-based model to a phase-retrieved interface in a PB-PCXI tomographic reconstruction, which is obtained when Paganin-type phase-retrieval is applied with incorrect values of $\delta$ and $\beta$. The fit parameters can then be used to calculate true $\delta$ and $\beta$ values for composite materials. This approach requires no a priori sample information, making it broadly applicable. Our PB-PCXI reconstruction is single distance, requiring only one exposure per tomographic angle, which is important for radiosensitive samples. We apply this approach to a breast-tissue sample, recovering the refraction component, $\delta$, with 0.6 - 2.4\% accuracy compared to theoretical values.

Ghost Projection

Ghost imaging is a developing imaging technique that employs random masks to image a sample. Ghost projection utilizes ghost-imaging concepts to perform the complementary procedure of projection of a desired image. The key idea underpinning ghost projection is that any desired spatial distribution of radiant exposure may be produced, up to an additive constant, by spatially-uniformly illuminating a set of random masks in succession. We explore three means of achieving ghost projection: (i) weighting each random mask, namely selecting its exposure time, according to its correlation with a desired image, (ii) selecting a subset of random masks according to their correlation with a desired image, and (iii) numerically optimizing a projection for a given set of random masks and desired image. The first two protocols are analytically tractable and conceptually transparent. The third is more efficient but less amenable to closed-form analytical expressions. A comparison with existing image-projection techniques is drawn and possible applications are discussed. These potential applications include: (i) a data projector for matter and radiation fields for which no current data projectors exist, (ii) a universal-mask approach to lithography, (iii) tomographic volumetric additive manufacturing, and (iv) a ghost-projection photocopier.