Due to the scarcity of spectrum resources, the emergence of new technologies and ever-increasing number of wireless devices operating in the radio frequency spectrum lead to data congestion and interference. In this work, we study the effect of altitude on sub-6 GHz spectrum measurement results obtained at a Helikite flying over two distinct scenarios; i.e., urban and rural environments. Specifically, we aim at investigating the spectrum occupancy of various long-term evolution (LTE), $5^{\text{th}}$ generation (5G) and citizens broadband radio service (CBRS) bands utilized in the United States for both uplink and downlink at altitudes up to 180 meters. Our results reveal that generally the mean value of the measured power increases as the altitude increases where the line-of-sight links with nearby base stations is more available. SigMF-compliant spectrum measurement datasets used in this paper covering all the bands between 100~MHz to 6~GHz are also provided.