Recently different evolutionary computation approaches have been developed that generate sets of high quality diverse solutions for a given optimisation problem. Many studies have considered diversity 1) as a mean to explore niches in behavioural space (quality diversity) or 2) to increase the structural differences of solutions (evolutionary diversity optimisation). In this study, we introduce a co-evolutionary algorithm to simultaneously explore the two spaces for the multi-component traveling thief problem. The results show the capability of the co-evolutionary algorithm to achieve significantly higher diversity compared to the baseline evolutionary diversity algorithms from the the literature.