UMBRELLA is a large-scale, open-access Internet of Things (IoT) ecosystem incorporating over 200 multi-sensor multi-wireless nodes, 20 collaborative robots, and edge-intelligence-enabled devices. This paper provides a guide to the implemented and prospective artificial intelligence (AI) capabilities of UMBRELLA in real-world IoT systems. Four existing UMBRELLA applications are presented in detail: 1) An automated streetlight monitoring for detecting issues and triggering maintenance alerts; 2) A Digital twin of building environments providing enhanced air quality sensing with reduced cost; 3) A large-scale Federated Learning framework for reducing communication overhead; and 4) An intrusion detection for containerised applications identifying malicious activities. Additionally, the potential of UMBRELLA is outlined for future smart city and multi-robot crowdsensing applications enhanced by semantic communications and multi-agent planning. Finally, to realise the above use-cases we discuss the need for a tailored MLOps platform to automate UMBRELLA model pipelines and establish trust.