In this article, we introduce LLMind, an innovative AI framework that utilizes large language models (LLMs) as a central orchestrator. The framework integrates LLMs with domain-specific AI modules, enabling IoT devices to collaborate effectively in executing complex tasks. The LLM performs planning and generates control scripts using a reliable and precise language-code transformation approach based on finite state machines (FSMs). The LLM engages in natural conversations with users, employing role-playing techniques to generate contextually appropriate responses. Additionally, users can interact easily with the AI agent via a user-friendly social media platform. The framework also incorporates semantic analysis and response optimization techniques to enhance speed and effectiveness. Ultimately, this framework is designed not only to innovate IoT device control and enrich user experiences but also to foster an intelligent and integrated IoT device ecosystem that evolves and becomes more sophisticated through continuing user and machine interactions.