By increasing model parameters but activating them sparsely when performing a task, the use of Mixture-of-Experts (MoE) architecture significantly improves the performance of Large Language Models (LLMs) without increasing the inference cost. However, the memory consumption due to the growing number of experts presents a challenge to the deployment of these models in many real world settings. Our empirical study reveals that some experts encode redundant knowledge during pre-training. We thus propose a method of grouping and pruning similar experts to improve model's parameter efficiency. We validate the effectiveness of our method by pruning two state-of-the-art MoE models, Mixtral-8x7B and Mixtral-8x22B. Evaluation shows that our method outperforms other model pruning methods on a range of natural language tasks. To facilitate future research, we will release our code and the pruned MoE models.