Traditional archival practices for describing electronic theses and dissertations (ETDs) rely on broad, high-level metadata schemes that fail to capture the depth, complexity, and interdisciplinary nature of these long scholarly works. The lack of detailed, chapter-level content descriptions impedes researchers' ability to locate specific sections or themes, thereby reducing discoverability and overall accessibility. By providing chapter-level metadata information, we improve the effectiveness of ETDs as research resources. This makes it easier for scholars to navigate them efficiently and extract valuable insights. The absence of such metadata further obstructs interdisciplinary research by obscuring connections across fields, hindering new academic discoveries and collaboration. In this paper, we propose a machine learning and AI-driven solution to automatically categorize ETD chapters. This solution is intended to improve discoverability and promote understanding of chapters. Our approach enriches traditional archival practices by providing context-rich descriptions that facilitate targeted navigation and improved access. We aim to support interdisciplinary research and make ETDs more accessible. By providing chapter-level classification labels and using them to index in our developed prototype system, we make content in ETD chapters more discoverable and usable for a diverse range of scholarly needs. Implementing this AI-enhanced approach allows archives to serve researchers better, enabling efficient access to relevant information and supporting deeper engagement with ETDs. This will increase the impact of ETDs as research tools, foster interdisciplinary exploration, and reinforce the role of archives in scholarly communication within the data-intensive academic landscape.